| Mwaka | Filamu | Kama | Maelezo |
|---|
| 1965 | Three Rooms in Manhattan | Client at the diner | |
| 1968 | Greetings | Jon Rubin | |
| 1969 | Sam's Song | Sam | |
| The Wedding Party | Cecil | |
| 1970 | Bloody Mama | Lloyd Barker | |
| Hi, Mom! | Jon Rubin | |
| 1971 | Jennifer on My Mind | Mardigian, Cab driver | |
| Born to Win | Officer Danny | |
| The Gang That Couldn't Shoot Straight | Mario Trantino | |
| 1973 | Bang the Drum Slowly | Bruce Pearson | New York Film Critics Circle Award for Best Supporting Actor |
| Mean Streets | John 'Johnny Boy' Civello | National Society of Film Critics Award for Best Supporting Actor
Sant Jordi Awards — win |
| 1974 | The Godfather Part II | Vito Corleone | Academy Award for Best Supporting Actor |
| 1976 | Taxi Driver | Travis Bickle | |
| 1900 | Alfredo Berlinghieri | Sant Jordi Awards — win |
| The Last Tycoon | Monroe Stahr | Sant Jordi Awards — win |
| 1977 | New York, New York | Jimmy Doyle | Sant Jordi Awards — win |
| 1978 | The Deer Hunter | Michael Vronsky | |
| 1980 | Raging Bull | Jake LaMotta | Academy Award for Best Actor
Golden Globe Award for Best Actor – Motion Picture Drama
National Board of Review Award for Best Actor
New York Film Critics Circle Award for Best Actor
Boston Society of Film Critics Award for Best Actor
|
| 1981 | True Confessions | Monsignor Desmond "Des" Spellacy | |
| 1983 | The King of Comedy | Rupert Pupkin | |
| 1984 | Once Upon a Time in America | David "Noodles" Aaronson | Sant Jordi Awards - Win |
| Falling in Love | Frank Raftis | Sant Jordi Awards - win |
| 1985 | Brazil | Archibald 'Harry' Tuttle | |
| 1986 | The Mission | Rodrigo Mendoza | |
| 1987 | Angel Heart | Louis Cypher | |
| The Untouchables | Al Capone | |
| 1988 | Midnight Run | Jack Walsh | |
| 1989 | Jacknife | Joseph 'Jacknife' Megessey | |
| We're No Angels | Ned | |
| 1990 | Stanley & Iris | Stanley Everett Cox | |
| Goodfellas | James "Jimmy" Conway | New York Film Critics Circle Award for Best Actor |
| Awakenings | Leonard Lowe | National Board of Review Award for Best Actor
New York Film Critics Circle Award for Best Actor |
| 1991 | Guilty by Suspicion | David Merrill | |
| Backdraft | Donald 'Shadow' Rimgale | |
| Cape Fear | Maximilian "Max" Cady | |
| 1992 | Night and the City | Harry Fabian | |
| Mistress | Evan M. Wright | |
| 1993 | A Bronx Tale | Lorenzo Anello | |
| Mad Dog and Glory | Wayne 'Mad Dog' Dobie | |
| This Boy's Life | Dwight Hansen | |
| 1994 | Mary Shelley's Frankenstein | The Creature | |
| 1995 | A Hundred and One Nights | Le mari de la star-fantasme en croisière | |
| Casino | Sam 'Ace' Rothstein | |
| Heat | Neil McCauley | |
| 1996 | The Fan | Gilbert "Gil" Renard | |
| Sleepers | Father Bobby | |
| Marvin's Room | Dr. Wally | |
| 1997 | Cop Land | Lt. Moe Tilden | |
| Jackie Brown | Louis Gara | |
| Wag the Dog | Conrad Brean | |
| 1998 | Great Expectations | Arthur Lustig | |
| Ronin | Sam | |
| 1999 | Analyze This | Paul Vitti | |
| Flawless | Walter Koontz | |
| 2000 | The Adventures of Rocky and Bullwinkl] | Fearless Leader | |
| Men of Honor | Chief Leslie William 'Billy' Sunday | |
| Meet the Parents | Jack Tiberius Byrnes | |
| 2001 | 15 Minutes | Det. Eddie Flemming | |
| The Score | Nick Wells | |
| 2002 | Showtime | Det. Mitch Preston | |
| City by the Sea | Vincent Anthony LaMarca | |
| Analyze That | Paul Vitti | |
| 2004 | Godsend | Dr. Richard Wells | |
| Shark Tale | Don Lino | Sauti |
| Meet the Fockers | Jack Tiberius Byrnes | |
| The Bridge of San Luis Rey | Archbishop of Lima | |
| 2005 | Hide and Seek | David Callaway / Charlie | |
| 2006 | Arthur and the Invisibles | The King | Sauti |
| The Good Shepherd | General Bill Sullivan | |
| 2007 | Stardust | Captain Shakespeare | |
| 2008 | Righteous Kill | Det. Thomas "Turk" Cowan | |
| What Just Happened | Ben | |
| 2009 | Everybody's Fine | Frank | Hollywood Film Festival Best Actor |
| 2010 | Machete | Senator McLaughlin | |
| Stone | Jack Mabry | |
| Little Fockers | Jack Tiberius Byrnes | |
| 2011 | Manuale d'amore 3 | Adrian | |
| Killer Elite | Hunter | |
| Limitless | Carl Van Loon | |
| New Year's Eve | Stan Harris | |
| 2012 | Being Flynn | Jonathan Flynn | |
| Red Lights | Simon Silver | |
| Freelancers | Sarcone | |
| The Big Wedding | Don Griffin | |
| The Silver Linings Playbook | Patrick Peoples | |
| 2013 | The Comedian | Jackie Burke | |
| Killing Season | Benjamin Ford | |
| Hands of Stone | Ray Arcel | |
