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US3800812A - Dental floss and method of making same - Google Patents

Dental floss and method of making same
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US3800812A
US3800812AUS00309878AUS3800812DAUS3800812AUS 3800812 AUS3800812 AUS 3800812AUS 00309878 AUS00309878 AUS 00309878AUS 3800812D AUS3800812D AUS 3800812DAUS 3800812 AUS3800812 AUS 3800812A
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dental floss
molecular weight
psi
tape
elastomer
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US00309878A
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P Jaffe
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Pauldan Ind Inc
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Pauldan Ind Inc
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Abstract

A polyester elastomer is extruded into a hot and tacky tape having certain tensile properties when cooled, including a high degree of stretchability; and by subsequent stretching of the cooled product, its break strength is substantially increased while it develops desirable elastomeric properties. The tape is cut into strips of dental floss of 1- 1/2 to 10 mils thickness either before or after the stretching, and abrasive particles and a flavoring agent may be incorporated into the tape material or applied to the tape surface.

Description

United States Patent Jaffe 1 Apr. 2, 1974 1 DENTAL FLOSS AND METHOD OF 3,511,249 5 1970 Baitz 132/89 MAKING SAME 2,381,142 8/1945 Stonehill 132/89 [75] Inventor: Paul E. Jaffe, Scarsdale, NY. Primary Examiner RuSSe" R. Kinsey [73] Assignee: Pauldan Industries, Inc., New York, Assis ant Examiner-Gregory E. MCNeill NY. 22 Filed: Nov. 27, 1972 [57] ABSTRACT A polyester elastomer is extruded into a hot and tacky [21] App! 309878 tape having certain tensile properties when cooled, including a high degree of stretchability; and by subse- [52] 11.8. C1. 132/89 qu n stretching of the cooled p i break [51] Int. Cl. A6lc 15/00 ng h is tan i lly increa ed while it develops de- [58] Field of Search 132/89, 90, 91; 424/67; sirable elastomeric properties. The tape is cut into 167/93 strips of dental floss of 1-% to 10 mils thickness either before or after the stretching, and abrasive particles [56] References Cited and a flavoring agent may be incorporated into the UNITED STATES PATENTS tape material or applied to the tape surface.
1 1954 Ashton 167/93 13 Claims, No Drawings DENTAL FLOSS AND METHOD OF MAKING SAME This invention relates to dental floss and more particularly to an improved dental floss which, as compared to conventional products of this type, is softer and more gentle in its tooth cleansing action and yet is more effective for cleaning interproximal tooth surface areas.
Toothbrushes are not suited for penetrating the restricted regions between closely adjacent teeth. Accordingly, it is common practice to use dental floss to supplement toothbrushing, in order to remove food particles held between the teeth. However, conventional dental floss has several objectionable features inhering from its construction, which consists of multistrand yarns coated with a wax-like substance. For example, it is quite resistant to deformation of its crosssectional area, so that it is poorly adapted to accommodate variations in inter-tooth contact pressures; and it provides a harsh cleansing action at best.
The principal object of the present invention is to provide a dental floss which eliminates these objectionable features and which is well suited to incorporate a flavoring agent and/or mild abrasive material.
A dental floss made according to the invention comprises a strip of elastomer, preferably polyester elastomer, with a thickness of 1-% to mils and having the following tensile properties:
a. Modulus of elasticity in tension, in the longitudinal direction, of 4,000 to 10,000 psi, preferably 5,000 to 6,000 psi.
b. Minimum break strength of 7,000 psi, preferably 1 1,500 to 14,000 psi.
c. Ultimate elongation of 200 to 1,000 percent, preferably 275 to 350 percent.
1 have found that in the use of a dental floss with these characteristics, it does not stretch excessively or break and yet is readily deformable in cross-section so that it can quite easily enter inter-tooth regions which are difficult to reach with conventional dental floss. Moreover, it provides a gentle cleansing action which is highly effective regardless of variations in the intertooth contact pressures or clearances, because upon reduction of the relatively high tension to which it is subjected when applying it between teeth, it tends to expand more or less against the adjacent teeth surfaces, depending upon the amount of such contact pressure or clearance.
The elastomer may be of various kinds. Polyester elastomer is preferred, but other examples are silicon polycarbonates, styrene butadienes, styrene ethylene propylenes; polypropylenes and thermoplastic polyurethanes. l have found that an elastomer particularly well suited for the new dental floss is a polyester elastomer sold by Du Font and known as Hytrel, which is a polycondensation product made by condensing at least one aromatic dicarboxylic acid or its ester having a molecular weight below 300 with a polyalkylene ether glycol having a molecular weight of 400 to 6,000 and at least one diol having a molecular weight below 250.
Preferably the new dental floss is made from the Bytrel elastomer which is sold by Du Pont as Hytrel 4055. This material may be extruded into film which is unstretched and which has the following tensile properties when cooled to room temperature:
a. Modulus of elasticity in tension in the order of 5,300 to 5,700 psi. b. Break strength in the order of 7,200 to 7,500 psi.
c. Ultimate elongation in the order of 750 to 850 percent.
d. No significant yield.
To provide this fllm with the preferred properties of the new dental floss, it is stretched longitudinally (i.e., in the direction in which it was extruded) approximately 350 percent, thereby modifying these properties to the following values:
a. Modulus of elasticity in tension, in the longitudinal direction, in the order of 5,300 to 5,700 psi.
b. Break strength in the order of 11,500 to 14,000
0. Ultimate elongation in the order of 300 to 350 percent.
d. No significant yield.
In the preferred embodiment of the invention, the strip of elastomer dental floss is provided with a pulverized abrasive and a flavoring agent. The latter may be incorporated in the elastomer before or during its extrusion into film or by coating the extruded film. These abrasive and flavoring additives may be a conventional tooth powder and are preferably sprayed upon a film or tape of the elastomer while it is still hot and tacky from the extruder which forms it, although the additives may be applied to the film or tape while it is reheated after being extruded and cooled. After cooling of the extruded film or tape (hereinafter referred to collectively as tape), it is cut into strips of dental floss having the aforementioned thickness of 1- /2 to 10 mils. In cases where the tape must be stretched to provide it with the tensile properties according to the invention (as in the case of Hytrel 4055 film), the stretching may be effected between the cooling and cutting steps or after the cutting step.
An example of the pulverized abrasive additive is calcium carbonate having a particle size of 0.1 to 2.0 microns, which may be added in an amount constituting about three percent by weight of the dental floss strip. Examples of the flavoring agent are peppermint oil, Spearmint oil and Wintergreen oil, and it may be added in any desired amount.
The elastomer forming the new dental floss preferably has a tack temperature above 200F (the tack temperature of the Hytrel 4055 tape being about 230-235F). This enables it to become sufficiently tacky from the heat of extrusion of the tape so that the additives will become firmly embedded in the tape surfaces after cooling and will remain firmly embedded in the uncut surfaces of the dental floss strips under normal conditions.
The abrasive additive serves as an aid in cleansing between teeth. As an alternative, however, the surfaces of the tape may be roughened prior to cutting of the strips of dental floss, as by sand-blasting or stippling or by rolling impressions on the surfaces.
The new dental floss may have any desired crosssectional configuration, such as round, oval, square or rectangular; and it will be understood that the thickness dimension of l-% to 10 mils applies to the diameter of a round configuration, to the spacing between opposing sides of a square configuration, and to the minimum spacing between opposing sides of an oval or rectangular configuration. Preferably, the cross-section is a rectangular one having a maximum dimension (width) of H16 to Ms inch.
cent of original length at which break occurs in the tensile test.
As previously mentioned, the Hytrel 4055 elastomer is particularly well suited for the manufacture of the new dental floss. This elastomer in the unstretched form behaves like a plastic material in that it has a distinct yield point in tension. The elongation at the yield point is considerably below 350 percent. In stretching to 350 percent, the material is therefore stressed beyond its yield point and permanent elongation takes place. Because the tensile strength beyond the yield point is so much greater than the yield strength, the permanent elongation is substantially unifonn throughout the length of the specimen. This is an unusual property for a material to possess at room temperature, which apparently contributes significantly to the success of the material for use as dental floss according to the invention. In the region on the stress-strain curve between the yield point and failure, that is, in the stretched form, the material can be said to behave like an elastomer. As is characteristic of elastomers, there is no apparent yield point in this region.
I claim:
1. A dental floss comprising a strip of elastomer with a thickness of l-% to mils, said strip having the following tensile properties:
a. Modulus of elasticity in tension, in the longitudinal direction, of 4,000 to 10,000 psi.
b. Minimum break strength of 7,000 psi.
c. Ultimate elongation of 200 to 1,000 percent.
2. A dental floss according to claim 1, in which said modulus is 5,000 to 6,000 psi, the break strength is 11,500 to 14,000 psi, and the ultimate elongation is 275 to 350 percent.
3. A dental floss according to claim 2, in which said elastomer is a polyester which is a polycondensation product made by condensing at least one aromatic dicarboxylic acid or its ester having a molecular weight below 300 with a polyalkylene ether glycol having a molecular weight of 400 to 6,000 and at least one diol having a molecular weight below 250.
4. A dental floss according to claim 1, in which said strip has a tack temperature above 200F.
5. A dental floss according to claim 1, comprising also a flavoring agent carried by said strip.
6. A dental floss according to claim 1, comprising also a pulverized abrasive material carried by said strip.
7. A dental floss according to claim 6, in which said abrasive material has a particle size of 0.1 to 2.0 microns and constitutes about 3 percent by weight of the strip.
8. A method of making dental floss, which comprises extruding a polyester elastomer into a hot and tacky tape which, when cooled, is untacky and has the following tensile properties:
a. Modulus of elasticity in tension in the order of 5,300 to 5,700 psi. b. Break strength in the order of 7,200 to 7,500 psi. 0. Ultimate elongation in the order of 750 to 850 percent, cooling the extruded tape, cutting the tape into strips having a thickness of l-% to 10 mils, and stretching the material from one of said cooling and cutting steps to increase said break strength to about 11,500 to 14,000 psi, thereby reducing said ultimate elongation to about 300 to 350 percent.
9. A method according to claim 8, in which said elastomer is a polycondensation product made by condensing at least one aromatic dicarboxylic acid or its ester having a molecular weight below 300 with a polyalkylene ether glycol having a molecular weight of 400 to 6,000 and at least one diol having a molecular weight of 400 to 6,000 and at least one diol having a molecular weight below 250.
10. A method according to claim 8, comprising also the step of applying a pulverized abrasive material to said polyester elastomer.
11. A method according to claim 8, comprising also the step of applying a flavoring agent to said polyester elastomer.
12. A method according to claim 8, in which said stretching is effected after said cooling but prior to said cutting.
13. The method of claim 8, in which said stretching is effected after said cutting.

Claims (12)

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Cited By (56)

* Cited by examiner, † Cited by third party
Publication numberPriority datePublication dateAssigneeTitle
US3943949A (en)*1974-11-261976-03-16Johnson & JohnsonFlavored dental articles
US3957067A (en)*1975-04-161976-05-18Ferraro Kenneth NDurable dental floss
US3985147A (en)*1975-03-131976-10-12Ricketts Craig MDental implement for removing stains from teeth
US4033365A (en)*1976-01-231977-07-05Johnson & JohnsonFlavored dental articles
EP0028130A1 (en)*1979-10-261981-05-06Peter Donald Wallace BirchTooth cleaning aids
US4836226A (en)*1987-11-201989-06-06Wolak Ronald GEndless article for cleaning teeth
EP0292673A3 (en)*1987-03-311989-11-23Toshiki TanakaElastic dental floss and holder for elastic dental floss with or without toothbrush
US4941487A (en)*1989-07-111990-07-17Vanbeneden Floyd VFluoridated dental floss
US4986289A (en)*1986-11-041991-01-22Mcwhorter Charles EPackaged pre-cut dental floss product
US5209251A (en)*1988-03-291993-05-11Colgate-Palmolive CompanyDental floss
US5226435A (en)*1991-08-011993-07-13Gillette Canada Inc.Flavored dental floss and method
WO1993015686A1 (en)*1992-02-061993-08-19Gillette Canada Inc.Improved flavored dental cleaning article and method
US5433226A (en)*1994-03-091995-07-18Delta Dental Hygienics, L.L.C.Dental floss based on robust segmented elastomer
EP0686390A2 (en)1994-06-061995-12-13JOHNSON & JOHNSON CONSUMER PRODUCTS, INC.Novel compositions for dental floss
US5479952A (en)*1994-01-061996-01-02Polteco, Inc.Dental floss of ultra-high modulus line material with enhanced mechanical properties
US5680876A (en)*1995-06-011997-10-28Gillette Canada Inc.Floss brush manufacture and product
US5692530A (en)*1995-09-211997-12-02Anchor Advance Products, Inc.Braided dental floss
WO1998017197A1 (en)1996-10-241998-04-30Gillette Canada Inc.Particulate modified elastomeric flosses
WO1998050607A1 (en)*1997-05-071998-11-12Peri-Dent LimitedPlastics materials yarn
US5875797A (en)*1995-06-061999-03-02Gillette Canada Inc.Dental floss
US6003525A (en)*1998-03-141999-12-21Katz; Harry S.Elastomer floss and related flossing devices
AU714692B2 (en)*1994-06-062000-01-06Johnson & Johnson Consumer Companies, Inc.Novel compositions for dental floss
WO2000009034A1 (en)*1998-08-172000-02-24Athena Nordic AbExtensible polishing mono-filament dental floss
US6039054A (en)*1998-09-232000-03-21Gillette Canada CompanyDental floss
US6220256B1 (en)1997-10-272001-04-24Gore Enterprise Holdings, Inc.Dental floss holder and improved dental floss
US6270890B1 (en)1988-03-292001-08-07Colgate-Palmolive CompanyDental floss
US6293287B1 (en)1996-09-132001-09-25Gillette Canada Inc.UV-cured resin-coated dental floss
US6303063B1 (en)1999-06-112001-10-16Peri-Dent LimitedProcess of making a yarn
US6340027B1 (en)1998-08-172002-01-22Athena Nordic AbExtensible polishing mono-filament dental floss
US6371133B1 (en)*1996-05-012002-04-16Loops, L.L.C.Variable-guage tooth-flossing loops
WO2002053059A2 (en)2000-12-292002-07-11Kimberly-Clark Worldwide, Inc.Hemostat coated dental floss and hemostat coated dental tape
US20020145066A1 (en)*2001-01-222002-10-10Michael SchweigertCoated monofilament tape bobbins and methods for winding
US6545077B2 (en)2000-08-232003-04-08International Tape Partners, LlcMonofilament dental tapes with substantive coatings
US6575176B1 (en)2001-08-232003-06-10International Tape Partners, LlcMonofilament dental tapes with soft abrasive coatings
US6582634B2 (en)1998-05-072003-06-24Peri-Dent LimitedProcess of making a yarn
US6591844B2 (en)2001-01-222003-07-15Peri-Deat LimitedElastomeric monofilament dental tapes
US20030134052A1 (en)*2000-06-292003-07-17Dave Vipul BhupendraElectrostatic impregnation of powders on substrates
US6604534B2 (en)2000-08-232003-08-12International Tape Partners, LlcPhysical improvements in coated monofilament dental tapes
US6609527B2 (en)2001-01-222003-08-26International Tape Partners, LlcNon-crystalline saliva-soluble coatings for elastomeric monofilament dental tapes
US20030168077A1 (en)*2002-02-112003-09-11Brown Dale G.Coated micromesh dental devices overcoated with imbedded particulate
US20030178044A1 (en)*2002-02-112003-09-25Brown Dale G.Micromesh interproximal devices
US20030200983A1 (en)*2001-08-232003-10-30Brown Dale G.Particulate coated monofilament devices
US20040123877A1 (en)*2002-12-302004-07-01Brown Dale G.Coated multifilament dental devices overcoated with imbedded particulate
US20050163825A1 (en)*2004-01-272005-07-28Naidu A. S.Lactoferrin-treated filament materials
US20050175551A1 (en)*2002-10-242005-08-11Heng CaiSilicon modified polyamide material useful for oral care
US7093417B1 (en)2005-04-042006-08-22Maczura David SMethod for making rope
US20060243297A1 (en)*2005-04-292006-11-02Brown Dale GCoated monofilament oriented HDPE dental tapes
WO2008074473A2 (en)2006-12-192008-06-26Basf SeUses and methods for preventing and/or treating caries caused by mutants streptococci
EP2133414A1 (en)2008-06-112009-12-16Basf SeUses and methods for preventing and /or treating oral malodour
EP2149632A1 (en)*2008-07-312010-02-03Mcneil-PPC, IncProcess for coating dental tape
US20100024838A1 (en)*2008-07-312010-02-04Harold OchsProcess for Winding Dental Tape
US20100024722A1 (en)*2008-07-312010-02-04Harold OchsApparatus for Coating Dental Tape
US20100024721A1 (en)*2008-07-312010-02-04Harold OchsApparatus for Coating Dental Tape
WO2012100991A1 (en)2011-01-242012-08-02Basf SeOral health improving compositions
US20140041681A1 (en)*2011-04-202014-02-13William EwingCompact, Recyclable, Multi-Layered Dental Flossing Device and Packaging Therefore
US20220161528A1 (en)*2020-11-242022-05-26Chance Line Industrial Co., Ltd.Filament made from cutting membrane material and being thinned to improve physical properties and manufacturing method thereof

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Cited By (83)

* Cited by examiner, † Cited by third party
Publication numberPriority datePublication dateAssigneeTitle
US3943949A (en)*1974-11-261976-03-16Johnson & JohnsonFlavored dental articles
US3985147A (en)*1975-03-131976-10-12Ricketts Craig MDental implement for removing stains from teeth
US3957067A (en)*1975-04-161976-05-18Ferraro Kenneth NDurable dental floss
US4033365A (en)*1976-01-231977-07-05Johnson & JohnsonFlavored dental articles
EP0028130A1 (en)*1979-10-261981-05-06Peter Donald Wallace BirchTooth cleaning aids
US4986289A (en)*1986-11-041991-01-22Mcwhorter Charles EPackaged pre-cut dental floss product
EP0292673A3 (en)*1987-03-311989-11-23Toshiki TanakaElastic dental floss and holder for elastic dental floss with or without toothbrush
US4836226A (en)*1987-11-201989-06-06Wolak Ronald GEndless article for cleaning teeth
US5209251A (en)*1988-03-291993-05-11Colgate-Palmolive CompanyDental floss
US6270890B1 (en)1988-03-292001-08-07Colgate-Palmolive CompanyDental floss
US4941487A (en)*1989-07-111990-07-17Vanbeneden Floyd VFluoridated dental floss
US5357990A (en)*1991-08-011994-10-25Gillette Canada Inc.Flavored dental floss and process
US5226435A (en)*1991-08-011993-07-13Gillette Canada Inc.Flavored dental floss and method
WO1993015686A1 (en)*1992-02-061993-08-19Gillette Canada Inc.Improved flavored dental cleaning article and method
US5353820A (en)*1992-02-061994-10-11Gillette Canada Inc.Flavored dental cleaning article and method
US5479952A (en)*1994-01-061996-01-02Polteco, Inc.Dental floss of ultra-high modulus line material with enhanced mechanical properties
WO1995024167A1 (en)*1994-03-091995-09-14Delta Dental Hygienics-LlcDental floss based on robust segmented elastomer
US5433226A (en)*1994-03-091995-07-18Delta Dental Hygienics, L.L.C.Dental floss based on robust segmented elastomer
EP0686390A2 (en)1994-06-061995-12-13JOHNSON & JOHNSON CONSUMER PRODUCTS, INC.Novel compositions for dental floss
EP0686390A3 (en)*1994-06-061996-07-24Johnson & Johnson Consumer New compositions for dental floss
AU714692B2 (en)*1994-06-062000-01-06Johnson & Johnson Consumer Companies, Inc.Novel compositions for dental floss
AU694983B2 (en)*1994-06-061998-08-06Johnson & Johnson Consumer Companies, Inc.Novel compositions for dental floss
US5680876A (en)*1995-06-011997-10-28Gillette Canada Inc.Floss brush manufacture and product
US5875797A (en)*1995-06-061999-03-02Gillette Canada Inc.Dental floss
US5692530A (en)*1995-09-211997-12-02Anchor Advance Products, Inc.Braided dental floss
US6371133B1 (en)*1996-05-012002-04-16Loops, L.L.C.Variable-guage tooth-flossing loops
US6293287B1 (en)1996-09-132001-09-25Gillette Canada Inc.UV-cured resin-coated dental floss
US6192896B1 (en)*1996-10-242001-02-27Gillette Canada CompanyParticulate modified elastomeric flosses
WO1998017197A1 (en)1996-10-241998-04-30Gillette Canada Inc.Particulate modified elastomeric flosses
AU733571B2 (en)*1996-10-242001-05-17Gillette Canada Inc.Particulate modified elastomeric flosses
US5918609A (en)*1996-10-241999-07-06Gillette Canada Inc.Particulate modified elastomeric flosses
WO1998050607A1 (en)*1997-05-071998-11-12Peri-Dent LimitedPlastics materials yarn
US6220256B1 (en)1997-10-272001-04-24Gore Enterprise Holdings, Inc.Dental floss holder and improved dental floss
US6003525A (en)*1998-03-141999-12-21Katz; Harry S.Elastomer floss and related flossing devices
US6582634B2 (en)1998-05-072003-06-24Peri-Dent LimitedProcess of making a yarn
US6340027B1 (en)1998-08-172002-01-22Athena Nordic AbExtensible polishing mono-filament dental floss
WO2000009034A1 (en)*1998-08-172000-02-24Athena Nordic AbExtensible polishing mono-filament dental floss
US6039054A (en)*1998-09-232000-03-21Gillette Canada CompanyDental floss
US6303063B1 (en)1999-06-112001-10-16Peri-Dent LimitedProcess of making a yarn
US6849303B2 (en)*2000-06-292005-02-01Vipul Bhupendra DaveMethod for electrostatically coating a fiber substrate
US20050008856A1 (en)*2000-06-292005-01-13Dave Vipul BhupendraMedical device having electrostatic coating with chemotherapeutic agents
US20030134052A1 (en)*2000-06-292003-07-17Dave Vipul BhupendraElectrostatic impregnation of powders on substrates
US6916880B2 (en)2000-08-232005-07-12International Tape Partners, LlcMonofilament dental tapes with substantive coatings
US6604534B2 (en)2000-08-232003-08-12International Tape Partners, LlcPhysical improvements in coated monofilament dental tapes
US6545077B2 (en)2000-08-232003-04-08International Tape Partners, LlcMonofilament dental tapes with substantive coatings
US20030225196A1 (en)*2000-08-232003-12-04International Tape Partners, LlcMonofilament dental tapes with substantive coatings
US6536448B2 (en)2000-12-292003-03-25Kimberly-Clark Worldwide, Inc.Hemostat coated dental floss and hemostat coated dental tape
WO2002053059A2 (en)2000-12-292002-07-11Kimberly-Clark Worldwide, Inc.Hemostat coated dental floss and hemostat coated dental tape
US6884309B2 (en)2001-01-222005-04-26International Tape Partners LlcCoated monofilament tape bobbins and methods for winding
US6609527B2 (en)2001-01-222003-08-26International Tape Partners, LlcNon-crystalline saliva-soluble coatings for elastomeric monofilament dental tapes
US20050226820A1 (en)*2001-01-222005-10-13Brown Dale GNon-crystalline saliva-soluble coatings for elastomeric monofilament dental tapes
US20050199334A1 (en)*2001-01-222005-09-15Michael SchweigertCoated monofilament tape bobbins and methods for winding
US6591844B2 (en)2001-01-222003-07-15Peri-Deat LimitedElastomeric monofilament dental tapes
US20040094181A1 (en)*2001-01-222004-05-20Brown Dale G.Non-crystalline saliva-soluble coatings for elastomeric monofilament dental tapes
US6907889B2 (en)2001-01-222005-06-21International Tape Partners, LlcNon-crystalline saliva-soluble coatings for elastomeric monofilament dental tapes
US20020145066A1 (en)*2001-01-222002-10-10Michael SchweigertCoated monofilament tape bobbins and methods for winding
US20060112968A1 (en)*2001-08-232006-06-01Brown Dale GParticulate coated monofilament devices
US6575176B1 (en)2001-08-232003-06-10International Tape Partners, LlcMonofilament dental tapes with soft abrasive coatings
US20030200983A1 (en)*2001-08-232003-10-30Brown Dale G.Particulate coated monofilament devices
US7017591B2 (en)2001-08-232006-03-28International Tape Partners LlcParticulate coated monofilament devices
US20030178044A1 (en)*2002-02-112003-09-25Brown Dale G.Micromesh interproximal devices
US7025986B2 (en)2002-02-112006-04-11International Tape Partners LlcMicromesh interproximal devices
US20030168077A1 (en)*2002-02-112003-09-11Brown Dale G.Coated micromesh dental devices overcoated with imbedded particulate
US20050175551A1 (en)*2002-10-242005-08-11Heng CaiSilicon modified polyamide material useful for oral care
US20040123877A1 (en)*2002-12-302004-07-01Brown Dale G.Coated multifilament dental devices overcoated with imbedded particulate
US7152611B2 (en)2002-12-302006-12-26International Tape Partners, LlcCoated multifilament dental devices overcoated with imbedded particulate
US20050163825A1 (en)*2004-01-272005-07-28Naidu A. S.Lactoferrin-treated filament materials
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