Ultrafast plasmonic nanowire lasers near the surface plasmon frequency
File(s)ultrafast-plasmonic-nanolasers.pdf (6.45 MB)
Accepted version
Author(s)
Type
Journal Article
Abstract
Light–matter interactions are inherently slow as the wavelengths of optical and electronic states differ greatly. Surface plasmon polaritons — electromagnetic excitations at metal–dielectric interfaces — have generated significant interest because their spatial scale is decoupled from the vacuum wavelength, promising accelerated light–matter interactions. Although recent reports suggest the possibility of accelerated dynamics in surface plasmon lasers, this remains to be verified. Here, we report the observation of pulses shorter than 800 fs from hybrid plasmonic zinc oxide (ZnO) nanowire lasers. Operating at room temperature, ZnO excitons lie near the surface plasmon frequency in such silver-based plasmonic lasers, leading to accelerated spontaneous recombination, gain switching and gain recovery compared with conventional ZnO nanowire lasers. Surprisingly, the laser dynamics can be as fast as gain thermalization in ZnO, which precludes lasing in the thinnest nanowires (diameter less than 120 nm). The capability to combine surface plasmon localization with ultrafast amplification provides the means for generating extremely intense optical fields, with applications in sensing, nonlinear optical switching, as well as in the physics of strong-field phenomena.
Date Issued
2014-11-01
Date Acceptance
2014-08-19
Citation
Nature Physics, 2014, 10 (11), pp.870-876
ISSN
1745-2473
Publisher
Nature Research
Start Page
870
End Page
876
Journal / Book Title
Nature Physics
Volume
10
Issue
11
Copyright Statement
© 2014 Macmillan Publishers Limited. All rights reserved.
Description
07.01.15 KB. OK to add accepted version to spiral, subject 6 months embargo
Identifier
http://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcApp=PARTNER_APP&SrcAuth=LinksAMR&KeyUT=WOS:000344846700022&DestLinkType=FullRecord&DestApp=ALL_WOS&UsrCustomerID=1ba7043ffcc86c417c072aa74d649202
Subjects
Science & Technology
Physical Sciences
Physics, Multidisciplinary
Physics
ENHANCED RAMAN-SCATTERING
WAVE-GUIDE
FLUORESCENCE
NANOLASER
THRESHOLD
ZNO
Publication Status
Published
Date Publish Online
2014-09-28