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Silicide

From Wikipedia, the free encyclopedia
Chemical compound that combines silicon and a more electropositive element
Structure oftitanium disilicide (Ti = white spheres).

Asilicide is a type ofchemical compound that combinessilicon and a usually moreelectropositive element.

Silicon is moreelectropositive thancarbon. In terms of their physical properties, silicides are structurally closer toborides than tocarbides. Because of size differences however silicides are not isostructural with borides and carbides.[1]

Bonds in silicides range fromconductive metal-like structures tocovalent orionic. Silicides of all non-transition metals have been described exceptberyllium. Silicides are used ininterconnects.[2]

Structure

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Silicon atoms in silicides can have many possible organizations:

  • Isolated silicon atoms: electrically conductive (or semiconductive)CrSi,MnSi,FeSi,CoSi,Cu5Si,(V,Cr,Mn)3Si,Fe3Si,Mn3Si,Mg2(Si,Ge,Sn,Pb),(Ca,Ru,Ce,Rh,Ir,Ni)2Si
  • Si2 pairs:U3Si2,hafnium andthorium silicides
  • Si4tetrahedra:KSi,RbSi,CsSi
  • Sin chains: USi,(Ti, Zr, Hf, Th, Ce, Pu)Si, CaSi, SrSi, YSi
  • Planar hexagonalgraphite-like Si layers: β-USi2, silicides of otherlanthanoids andactinoids
  • Corrugated hexagonal Si layers: CaSi2
  • Open three-dimensional Si skeletons: SrSi2, ThSi2, α-USi2

Preparation and reactivity

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Most silicides are produced by direct combination of the elements.[1]

A silicide prepared by a self-aligned process is called asalicide. This is a process in which silicide contacts are formed only in those areas in which deposited metal (which after annealing becomes a metal component of the silicide) is in direct contact with silicon, hence, the process is self-aligned. It is commonly implemented in MOS/CMOS processes for ohmic contacts of the source, drain, and poly-Si gate.

Alkali and alkaline earth metals

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Group 1 and 2 silicides e.g. Na2Si and Ca2Si react with water, yielding hydrogen and/or silanes.

Magnesium silicide reacts withhydrochloric acid to givesilane:

Mg2Si + 4 HCl → SiH4 + 2 MgCl2

Group 1 silicides are even more reactive. For example, sodium silicide, Na2Si, reacts rapidly with water to yieldsodium silicate, Na2SiO3, andhydrogen gas. Rubidium silicide ispyrophoric, igniting in contact with air.[3]

Transition metals and other elements

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Thetransition metal silicides are usually inert to aqueous solutions. At red heat, they react withpotassium hydroxide,fluorine, andchlorine.Mercury,thallium,bismuth, andlead areimmiscible with liquid silicon.

Applications

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Silicidethin films have applications in microelectronics due to their high electrical conductivity, thermal stability, corrosion resistance, and compatibility withphotolithographicwafer processes.[4] For example silicides formed over layers ofpolysilicon, calledpolycides, are commonly used as an interconnect material in integrated circuits for their high conductivity.[5] Silicides formed through the salicide process also see use as a lowwork function metal inohmic and Schottky contacts.[6] High work function metals are often not ideal for use in metal–semiconductor junctions directly due tofermi–level pinning where the Schottky barrier potential of the junction becomes locked around 0.7–0.8V. For this reason low forward-voltage Schottky diodes and ohmic interconnects between a semiconductor and a metal often utilize a thin layer of silicide at the metal–semiconductor interface.

List (incomplete)

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See also

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References

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  1. ^abGreenwood, Norman N.; Earnshaw, Alan (1997).Chemistry of the Elements (2nd ed.).Butterworth-Heinemann. p. 335-336.ISBN 978-0-08-037941-8.
  2. ^Schlesinger, Mark E. (1990). "Thermodynamics of solid transition-metal silicides".Chemical Reviews.90 (4):607–628.doi:10.1021/cr00102a003.
  3. ^Rubidium ampoule opened IN AIR for chemical reactions (Video). ChemicalForce. 22 Feb 2020. Event occurs at 10:51.Archived from the original on 2021-12-21. Retrieved2020-02-23.
  4. ^Murarka, Shayam (1995)."Silicide thin films and their applications in microelectronics".Intermetallics.3 (3):173–186.doi:10.1016/0966-9795(95)98929-3. Retrieved26 July 2023.
  5. ^Z. Ma, L. H. Allen (2004). "3.3 Fundamental aspects of Ti/Si thin film reaction". In L.J. Chen (ed.).Silicide Technology for Integrated Circuits (Processing). IET. pp. 50–61.ISBN 9780863413520.
  6. ^Monch, W. (1987).Role of virtual gap states and defects in metal-semiconductor contacts. Vol. 58. Physics Review Letter. pp. 1260–1263.doi:10.1103/PhysRevLett.58.1260.
Salts and covalent derivatives of thesilicide ion
SiH4
+H
He
LiSiBe2SiSiB3
SiB6
+B
SiC
+C
Si3N4
-N
+N
SiO2SiF4Ne
NaSiMg2SiAlSi4−SiP, SiP2
-P
+P
SiS2
-S
SiCl4Ar
KSiCaSi
CaSi2
ScSi Sc5Si3 Sc2Si3 Sc5Si4TiSi
TiSi2
V3Si V5Si3, V6Si5, VSi2, V6Si5Cr3Si Cr5Si3, CrSi, CrSi2MnSi,MnSi2, Mn9Si2, Mn3Si,Mn5Si3, Mn11Si9FeSi2
FeSi
Fe5Si3
Fe2Si
Fe3Si
CoSi,CoSi2,Co2Si, Co3SiNiSi,more…Cu17Si3, Cu56Si11, Cu5Si, Cu33Si7, Cu4Si, Cu19Si6, Cu3Si, Cu87Si13ZnGaGeSi
+Ge
SiAs, SiAs2
-As
+As
SiSe2 SiSeSiBr4Kr
RbSiSrSi2YSi Y5Si3, Y5Si4, Y3Si5, YSi1.4ZrSi Zr5Si3, Zr5Si4,ZrSi2, Zr3Si2, Zr2Si, Zr3SiNb4Si Nb5Si3MoSi2
Mo3Si Mo5Si3
TcRuSi Ru2Si, Ru4Si3, Ru2Si3RhSi Rh2Si, Rh5Si3, Rh3Si2, Rh20Si13PdSi Pd5Si, Pd9Si2, Pd3Si, Pd2SiAgCdInSnSbTeSi2 Te2Si3SiI4Xe
CsSiBa2Si BaSi2, Ba5Si3 Ba3Si4*Lu5Si3HfSi Hf2Si, Hf3Si2, Hf5Si4, HfSi2Ta9Si2, Ta3Si, Ta5Si3WSi2 W5Si3ReSi Re2Si, ReSi1.8 Re5Si3OsSiIrSiPtSiAuHgTlPbBiPoAtRn
FrRa**LrRfDbSgBhHsMtDsRgCnNhFlMcLvTsOg
 
*LaSi2 La5Si3, La3Si2, La5Si4, LaSiCeSi2 Ce5Si3, Ce3Si2, Ce5Si4,CeSi, Ce3Si5PrSi2 Pr5Si3, Pr3Si2, Pr5Si4, PrSiNdSi Nd5Si3, Nd5Si4, Nd5Si3, Nd3Si4, Nd2Si3, NdSixPmSmSi2 Sm5Si4, Sm5Si3, SmSi, Sm3Si5Eu?GdSi2 Gd5Si3, Gd5Si4, GdSiTbSi2 SiTb, Si4Tb5, Si3Tb5DySi2 DySiHoSi2 Ho5Si3, Ho5Si4, HoSi, Ho4Si5ErSi2 Er5Si3, Er5Si4, ErSiTm?YbSi Si1.8Yb, Si5Yb3, Si4Yb3, Si4Yb5, Si3Yb5
**AcThSiPaSiUSi2NpSi2PuSiAmCmBkCfEsFmMdNo
Group 1
Group 13
Group 14
Group 15 (Pnictides)
Group 16 (Chalcogenides)
Group 17 (Halides)
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