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Plumbide

From Wikipedia, the free encyclopedia
Compound containing a plumbide anion
Plumbide
[Pb5]2−

Plumbide is an anion oflead atoms. There are three plumbide anions, written as Pb, Pb2− and Pb4− with 3oxidation states, -1, -2 and -4, respectively.Aplumbide can refer to one of two things: anintermetallic compound that containslead, or aZintl phase compound with lead as the anion.

Zintl phase

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[Pb9]4− from [K(18-crown-6)]2K2Pb9·(en)1.5

Plumbides can be formed when lead forms a Zintl phase compound with a more metallic element. One salt that can be formed this way is whencryptand reacts withsodium and lead inethylenediamine (en) to produce[Na(crypt)]+
2
[Pb5]2−, which is red in solution.[1]Lead can also create anions withtin, in a series of anions with the formula [Sn9−xPbx]4−.

Lead can also form the [Pb9]4− anion, which is emerald green in solution.[2]

Examples

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An example of a plumbide is CeRhPb. The lead atom has acoordination number of 12 in the crystal structure of this compound. It is bound to fourrhodiums, sixceriums, and two other lead atoms in the crystal structure of the chemical.[3]

Several other plumbides are the M2Pd2Pb plumbides, where M is arare-earth element, and the intermetallic additionally contains apalladium. These plumbides tend to exhibit antiferromagnetism, and all of them are conductors.[4]

A third plumbide is Ti6Pb4.8. Like the above plumbides, it is an intermetallic, but it only containstitanium as the other metal, and not any rare earths.[5]

Plumbides can also beZintl phase compounds, such as [K(18-crown-6)]2K2Pb9·(en)1.5. This is not a simple Zintl compound, but rather contains the organic molecules18-crown-6 andethylenediamine (en) in order to stabilize the crystal structure.[6]

References

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  1. ^P. A. Edwards, J. D. Corbett (1977). "Stable homopolyatomic anions. Synthesis and crystal structures of salts containing the pentaplumbide(2−) and pentastannide(2−) anions".Inorg. Chem.16 (4):903–907.doi:10.1021/ic50170a036.
  2. ^Greenwood, Norman N.; Earnshaw, Alan (1997).Chemistry of the Elements (2nd ed.).Butterworth-Heinemann. pp. 391–396.ISBN 978-0-08-037941-8.
  3. ^Gulay, L. D.; D. Kaczorowskia; A. Szajekc; A. Pietraszkoa (August 2008)."Crystal and electronic structure and magnetic properties of CeRhPb"(PDF).Journal of Physics and Chemistry of Solids.69 (8). Elsevier:1934–1939.Bibcode:2008JPCS...69.1934G.doi:10.1016/j.jpcs.2008.01.020.S2CID 95282795.
  4. ^Kaczorowski, D.; L. D. Gulay (13 September 2007). "Magnetic and electrical properties of RE2Pd2Pb (RE = Y, La–Sm, Gd–Tm) compounds".Journal of Alloys and Compounds.442 (1–2). Elsevier:169–171.doi:10.1016/j.jallcom.2006.08.351.
  5. ^Kleinke, Holger (June 2001). "Extraordinarily Short Pb–Pb Bonds in the New Binary Intermetallic Ti6Pb4.8".Journal of Solid State Chemistry.159 (1). Academic Press:134–138.Bibcode:2001JSSCh.159..134K.doi:10.1006/jssc.2001.9141.
  6. ^Yong, Li; Stephan D. Hoffmann; Thomas F. Fässler (1 December 2006). "A low-dimensional arrangement of [Pb9]4− clusters in [K(18-crown-6)]2K2Pb9·(en)1.5".Inorganica Chimica Acta.359 (15). Elsevier:4774–4778.doi:10.1016/j.ica.2006.04.017.
Group 1
Group 13
Group 14
Group 15 (Pnictides)
Group 16 (Chalcogenides)
Group 17 (Halides)
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