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Wagner-Jauregg reaction

From Wikipedia, the free encyclopedia
Chemical reaction

TheWagner-Jauregg reaction is a classicorganic reaction inorganic chemistry, named afterTheodor Wagner-Jauregg [de] (son ofJulius Wagner-Jauregg), describing the doubleDiels–Alder reaction of 2 equivalents ofmaleic anhydride with a 1,1-diarylethylene. Afteraromatization of the bis-adduct, the ultimate reaction product is anaphthalene compound with onephenyl substituent.[1][2]

The reaction is unusual in that the anhydride reacts with the aromatic ring. The presence of the additional alpha-phenyl group on the phenylethene (the styryl group) activates the styryl for a Diels–Alder reaction even at the expense of its aromaticity. In contrast, unactivatedstyrene reacts instead at thealkene alone via a linear polymerization reaction.Styrene maleic anhydride copolymer is formed, retaining the aromaticity of the styrene.

The Diels–Alder product can be re-aromatized using elementalsulfur at high temperature, followed by a second rearomatization bydecarboxylation withbarium hydroxide andcopper:[3]

Wagner-Jauregg reaction
Wagner-Jauregg reaction

References

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  1. ^Theodor Wagner-Jauregg (1930). "Über addierende Hetero-polymerisation".Berichte der Deutschen Chemischen Gesellschaft (A and B Series).68 (11): 3218.doi:10.1002/cber.19300631140.
  2. ^Theodor Wagner-Jauregg (1931). "Die Addition von Maleinsäureanhydrid an asymm. Diphenyl-äthylen".Justus Liebig's Annalen der Chemie.491:1–13.doi:10.1002/jlac.19314910102.
  3. ^Felix Bergmann; Jacob Szmuszkowicz & George Fawaz (1947). "The Condensation of 1,1-Diarylethylenes with Maleic Anhydride".Journal of the American Chemical Society.69 (7):1773–1777.Bibcode:1947JAChS..69.1773B.doi:10.1021/ja01199a055.PMID 20251415.
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